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Suicune is a powerful legendary Pokémon that's part of a trio in Pokémon HeartGold and SoulSilver. Unlike its pals, Entei and Raikou, it doesn't randomly wander the map. Suicune will spawn in select places on the map; unmoving until you approach it. Since it's a quite elusive Pokémon, you need patience to capture it. Fortunately, the wild goose hunt to capture Suicune is well worth it. Read on from step one to find out how to find this awesome Pokémon.
Steps
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Fly, bike, or walk to Ecruteak City.
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At the top part of the city, there is a burned tower known as Brass Tower, or simply the Burned Tower. Enter it.Advertisement
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Walk to the right, then upwards. Climb down the ladder. Walk towards Suicune, Raikou, and Entei. They will run away.
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Go to Cianwood City. Walk north and you'll see Suicune again. Of course, it runs off, but you'll be able to catch it soon.
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Fly to either Ecruteak City and run right or Mahogany Town and run left. Either way gets you to Route 42. Go to the entrance of Mt. Mortar and you'll see Suicune again.
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Go through Mt. Silver to get to the Kanto region. Go to Vermillion City and you'll see it again.
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Go to Route 14. Don't worry, as this is the last time Suicune runs away.
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Bike or walk to Route 25. Go to Bill's (the creator of the Pokémon Storage System) house, and you'll see Suicune again. This time, it won't back off. Do a battle with Suicune.